Local elastic response measured near the colloidal glass transition.
نویسندگان
چکیده
We examine the response of a dense colloidal suspension to a local force applied by a small magnetic bead. For small forces, we find a linear relationship between the force and the displacement, suggesting the medium is elastic, even though our colloidal samples macroscopically behave as fluids. We interpret this as a measure of the strength of colloidal caging, reflecting the proximity of the samples' volume fractions to the colloidal glass transition. The strain field of the colloidal particles surrounding the magnetic probe appears similar to that of an isotropic homogeneous elastic medium. When the applied force is removed, the strain relaxes as a stretched exponential in time. We introduce a model that suggests this behavior is due to the diffusive relaxation of strain in the colloidal sample.
منابع مشابه
ar X iv : 1 21 0 . 35 86 v 1 [ co nd - m at . s of t ] 1 2 O ct 2 01 2 Local elastic response measured near the colloidal glass transition
We examine the response of a dense colloidal suspension to a local force applied by a small magnetic bead. For small forces, we find a linear relationship between the force and the displacement, suggesting the medium is elastic, even though our colloidal samples macroscopically behave as fluids. We interpret this as a measure of the strength of colloidal caging, reflecting the proximity of the ...
متن کامل5 N ov 2 00 1 Subdiffusion and the cage effect studied near the colloidal glass transition Eric
The dynamics of a glass-forming material slow greatly near the glass transition, and molecular motion becomes inhibited. We use confocal microscopy to investigate the motion of colloidal particles near the colloidal glass transition. As the concentration in a dense colloidal suspension is increased, particles become confined in transient cages formed by their neighbors. This prevents them from ...
متن کاملWeak correlations between local density and dynamics near the glass transition.
We perform experiments on two different dense colloidal suspensions with confocal microscopy to probe the relationship between local structure and dynamics near the glass transition. We calculate the Voronoi volume for our particles and show that this quantity is not a universal probe of glassy structure for all colloidal suspensions. We correlate the Voronoi volume to displacement and find tha...
متن کاملEffect of colloidal Particles associated with the liquid bridge in sticking during drying in Superheated Steam
It is very important in the design of a drying system is to evaluate sticking behaviour of the materials goes under drying. A new approach to the sticking issue is applied in this study by carrying out a sticking test for the liquid associated with the materials under study. It was found that the liquid bridge is responsible of the initial sticking of the materials to the contact surface and th...
متن کاملSubdiffusion and the cage effect studied near the colloidal glass transition
The dynamics of a glass-forming material slow greatly near the glass transition, and molecular motion becomes inhibited. We use confocal microscopy to investigate the motion of colloidal particles near the colloidal glass transition. As the concentration in a dense colloidal suspension is increased, particles become confined in transient cages formed by their neighbors. This prevents them from ...
متن کاملذخیره در منابع من
با ذخیره ی این منبع در منابع من، دسترسی به آن را برای استفاده های بعدی آسان تر کنید
عنوان ژورنال:
- The Journal of chemical physics
دوره 138 12 شماره
صفحات -
تاریخ انتشار 2013